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Dependence of Off-Diagonal Components of χ(3) on Substrate Temperature of Epitaxially Grown Vanadyl Phthalocyanine Films
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Single-crystalline vanadyl phthalocyanine films have been grown by the molecular beam epitaxy technique. The normalized off-diagonal ratio 3χ1221/χ1111 has been determined by circular-polarization third-harmonic generation measurement. It is revealed that the single-crystalline phase with 4mm symmetry can be distinguished from the C
∞υ polycrystalline phase by circular-polarization third-harmonic generation measurement, and the quality of the epitaxial film can be quantitatively analyzed by the normalized off-diagonal ratio of 3χ1221/χ1111.
Title: Dependence of Off-Diagonal Components of χ(3) on Substrate Temperature of Epitaxially Grown Vanadyl Phthalocyanine Films
Description:
Single-crystalline vanadyl phthalocyanine films have been grown by the molecular beam epitaxy technique.
The normalized off-diagonal ratio 3χ1221/χ1111 has been determined by circular-polarization third-harmonic generation measurement.
It is revealed that the single-crystalline phase with 4mm symmetry can be distinguished from the C
∞υ polycrystalline phase by circular-polarization third-harmonic generation measurement, and the quality of the epitaxial film can be quantitatively analyzed by the normalized off-diagonal ratio of 3χ1221/χ1111.
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